We present a detailed theoretical investigation of the linear and nonlinear optical response in a model system for a disordered d-wave superconductor. By evaluating the quasiparticle contribution (BCS response) we show that for both quantities the gap symmetry considerably changes the paradigm of the optical response as compared to the conventional s-wave case. For what concerns the linear response our findings agree with previous work showing that in strongly disordered d-wave superconductors a large fraction of uncondensed spectral weight survives below T-c, making the optical absorption around the gap-frequency scale almost unchanged with respect to the normal state. Our numerical results are in excellent quantitative agreement with experiments in overdoped cuprates. In the nonlinear regime we focus on the third-harmonic generation (THG), finding that, as already established for the s-wave case, in general a large THG is triggered by disorder-activated paramagnetic processes. However, in the d-wave case the BCS response is monotonously increasing in frequency, losing any signature of THG enhancement when the THz pump frequency omega matches the gap maximum Delta, a hallmark of previous experiments in conventional s-wave superconductors. Our findings, along with the mild polarization dependence of the response, provide an explanation for recent THG measurements in cuprates, setting the framework for the theoretical understanding of nonlinear effects in unconventional cuprates.

Linear and nonlinear current response in disordered d-wave superconductors / Benfatto, L.; Castellani, C.; Seibold, G.. - In: PHYSICAL REVIEW. B. - ISSN 2469-9950. - 108:13(2023), pp. 1-15. [10.1103/physrevb.108.134508]

Linear and nonlinear current response in disordered d-wave superconductors

Benfatto, L.
Primo
;
Castellani, C.
Secondo
;
Seibold, G.
Ultimo
2023

Abstract

We present a detailed theoretical investigation of the linear and nonlinear optical response in a model system for a disordered d-wave superconductor. By evaluating the quasiparticle contribution (BCS response) we show that for both quantities the gap symmetry considerably changes the paradigm of the optical response as compared to the conventional s-wave case. For what concerns the linear response our findings agree with previous work showing that in strongly disordered d-wave superconductors a large fraction of uncondensed spectral weight survives below T-c, making the optical absorption around the gap-frequency scale almost unchanged with respect to the normal state. Our numerical results are in excellent quantitative agreement with experiments in overdoped cuprates. In the nonlinear regime we focus on the third-harmonic generation (THG), finding that, as already established for the s-wave case, in general a large THG is triggered by disorder-activated paramagnetic processes. However, in the d-wave case the BCS response is monotonously increasing in frequency, losing any signature of THG enhancement when the THz pump frequency omega matches the gap maximum Delta, a hallmark of previous experiments in conventional s-wave superconductors. Our findings, along with the mild polarization dependence of the response, provide an explanation for recent THG measurements in cuprates, setting the framework for the theoretical understanding of nonlinear effects in unconventional cuprates.
2023
superconductors; non-linear optical response; disordered superconductors
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Linear and nonlinear current response in disordered d-wave superconductors / Benfatto, L.; Castellani, C.; Seibold, G.. - In: PHYSICAL REVIEW. B. - ISSN 2469-9950. - 108:13(2023), pp. 1-15. [10.1103/physrevb.108.134508]
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11573/1706083
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