Mechanical deformations and ensuing strain are routinely exploited to tune the band gap energy and to enhance the functionalities of two-dimensional crystals. In this Letter, we show that strain leads also to a strong modification of the exciton magnetic moment in WS2 monolayers. Zeeman-splitting measurements under magnetic fields up to 28.5 T were performed on single, one-layer-thick WS2 microbubbles. The strain of the bubbles causes a hybridization of k-space direct and indirect excitons resulting in a sizable decrease in the modulus of the g factor of the ground-state exciton. These findings indicate that strain may have major effects on the way the valley number of excitons can be used to process binary information in two-dimensional crystals.

Strain-Induced Exciton Hybridization in WS2 Monolayers Unveiled by Zeeman-Splitting Measurements / Blundo, E.; Junior, P. E. F.; Surrente, A.; Pettinari, G.; Prosnikov, M. A.; Olkowska-Pucko, K.; Zollner, K.; Wozniak, T.; Chaves, A.; Kazimierczuk, T.; Felici, M.; Babinski, A.; Molas, M. R.; Christianen, P. C. M.; Fabian, J.; Polimeni, A.. - In: PHYSICAL REVIEW LETTERS. - ISSN 0031-9007. - 129:6(2022). [10.1103/PhysRevLett.129.067402]

Strain-Induced Exciton Hybridization in WS2 Monolayers Unveiled by Zeeman-Splitting Measurements

Blundo E.;Surrente A.;Pettinari G.;Felici M.;Polimeni A.
2022

Abstract

Mechanical deformations and ensuing strain are routinely exploited to tune the band gap energy and to enhance the functionalities of two-dimensional crystals. In this Letter, we show that strain leads also to a strong modification of the exciton magnetic moment in WS2 monolayers. Zeeman-splitting measurements under magnetic fields up to 28.5 T were performed on single, one-layer-thick WS2 microbubbles. The strain of the bubbles causes a hybridization of k-space direct and indirect excitons resulting in a sizable decrease in the modulus of the g factor of the ground-state exciton. These findings indicate that strain may have major effects on the way the valley number of excitons can be used to process binary information in two-dimensional crystals.
2022
Excitons, transition metal dichalcogenides, magneto-optical spectroscopy
01 Pubblicazione su rivista::01a Articolo in rivista
Strain-Induced Exciton Hybridization in WS2 Monolayers Unveiled by Zeeman-Splitting Measurements / Blundo, E.; Junior, P. E. F.; Surrente, A.; Pettinari, G.; Prosnikov, M. A.; Olkowska-Pucko, K.; Zollner, K.; Wozniak, T.; Chaves, A.; Kazimierczuk, T.; Felici, M.; Babinski, A.; Molas, M. R.; Christianen, P. C. M.; Fabian, J.; Polimeni, A.. - In: PHYSICAL REVIEW LETTERS. - ISSN 0031-9007. - 129:6(2022). [10.1103/PhysRevLett.129.067402]
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11573/1652965
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