We demonstrate the control of enhanced chiral field distribution at the surface of hybrid metallo-dielectric nanostructures composed of self-assembled vertical hexagonal GaAs-based nanowires having three of the six sidewalls covered with Au. We show that weakly-guided modes of vertical GaAs nanowires can generate regions of high optical chirality that are further enhanced by the break of the symmetry introduced by the gold layer. Changing the angle of incidence of a linearly polarized plane wave it is possible to tailor and optimize the maps of the optical chirality in proximity of the gold plated walls. The low cost feasibility of the sample combined to the simple control by using linearly polarized light and the easy positioning of chiral molecules by functionalization of the gold plates make our proposed scheme very promising for enhanced enantioselective spectroscopy applications.
Chiral near-field manipulation in Au-GaAs hybrid hexagonal nanowires / Petronijevic, Emilija; Centini, Marco; Belardini, Alessandro; Leahu, Grigore; Hakkarainen, Teemu; Sibilia, Concetta. - In: OPTICS EXPRESS. - ISSN 1094-4087. - ELETTRONICO. - 25:13(2017), pp. 14148-14157. [10.1364/OE.25.014148]
Chiral near-field manipulation in Au-GaAs hybrid hexagonal nanowires
PETRONIJEVIC, EMILIJA;CENTINI, MARCO;BELARDINI, ALESSANDRO;LEAHU, GRIGORE;SIBILIA, Concetta
2017
Abstract
We demonstrate the control of enhanced chiral field distribution at the surface of hybrid metallo-dielectric nanostructures composed of self-assembled vertical hexagonal GaAs-based nanowires having three of the six sidewalls covered with Au. We show that weakly-guided modes of vertical GaAs nanowires can generate regions of high optical chirality that are further enhanced by the break of the symmetry introduced by the gold layer. Changing the angle of incidence of a linearly polarized plane wave it is possible to tailor and optimize the maps of the optical chirality in proximity of the gold plated walls. The low cost feasibility of the sample combined to the simple control by using linearly polarized light and the easy positioning of chiral molecules by functionalization of the gold plates make our proposed scheme very promising for enhanced enantioselective spectroscopy applications.File | Dimensione | Formato | |
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