We report on experiments which show that C60 can ionize in an indirect, quasi-thermal boiloff process after absorption of a single photon. The process involves a large number of incoherently excited valence electrons and yields electron spectra with a Boltzmann distribution with temperatures exceeding 10^4 K. It is expected to be present for other molecules and clusters with a comparatively large number of valence electrons. The astrophysical consequences are briefly discussed.
Single photon thermal ionization of C60 / Hansen, Klavs; Richter, Robert; Alagia, Michele; Stranges, Stefano; Schio, Luca; Salén, Peter; Yatsyna, Vasyl; Feifel, Raimund; Zhaunerchyk, Vitali. - In: PHYSICAL REVIEW LETTERS. - ISSN 0031-9007. - STAMPA. - 118:10(2017). [10.1103/PhysRevLett.118.103001]
Single photon thermal ionization of C60
STRANGES, Stefano;SCHIO, LUCA;
2017
Abstract
We report on experiments which show that C60 can ionize in an indirect, quasi-thermal boiloff process after absorption of a single photon. The process involves a large number of incoherently excited valence electrons and yields electron spectra with a Boltzmann distribution with temperatures exceeding 10^4 K. It is expected to be present for other molecules and clusters with a comparatively large number of valence electrons. The astrophysical consequences are briefly discussed.File | Dimensione | Formato | |
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