We present a systematic study of the low-energy electrodynamics of the magnetic FeSn kagome metal, which hosts both topological (Dirac) and non-trivial states. Our results reveal that the optical conductivity of FeSn shows two Drude contributions that can be associated with the linear (Dirac) and parabolic (massive) bands, with a dominance of the former to the DC conductivity at low temperatures. The weight of the Drude response shifts toward lower frequencies upon cooling due to a rapid increase in the Dirac electron mobility, which we associate with a temperature suppression of e–ph scattering. The experimental interband dielectric function is in very good agreement with that calculated within Density Functional Theory (DFT). These results provide a full description of the charge dynamics in FeSn kagome topological metal, opening the road for its use in photonic and plasmonic applications.

Evidence of high electron mobility in magnetic kagome topological metal FeSn thin films / Mosesso, Lorenzo; Tomarchio, Luca; Bhattarai, Niraj; Macis, Salvatore; Gori, Paola; Grilli, Antonio; Cestelli Guidi, Mariangela; Philip, John; Pulci, Olivia; Lupi, Stefano. - In: NANOSCALE ADVANCES. - ISSN 2516-0230. - (2024), pp. 1-8. [10.1039/d4na00737a]

Evidence of high electron mobility in magnetic kagome topological metal FeSn thin films

Mosesso, Lorenzo
;
Tomarchio, Luca;Macis, Salvatore
;
Lupi, Stefano
2024

Abstract

We present a systematic study of the low-energy electrodynamics of the magnetic FeSn kagome metal, which hosts both topological (Dirac) and non-trivial states. Our results reveal that the optical conductivity of FeSn shows two Drude contributions that can be associated with the linear (Dirac) and parabolic (massive) bands, with a dominance of the former to the DC conductivity at low temperatures. The weight of the Drude response shifts toward lower frequencies upon cooling due to a rapid increase in the Dirac electron mobility, which we associate with a temperature suppression of e–ph scattering. The experimental interband dielectric function is in very good agreement with that calculated within Density Functional Theory (DFT). These results provide a full description of the charge dynamics in FeSn kagome topological metal, opening the road for its use in photonic and plasmonic applications.
2024
kagome metals; IR and optical spectroscopy; quantum materials
01 Pubblicazione su rivista::01a Articolo in rivista
Evidence of high electron mobility in magnetic kagome topological metal FeSn thin films / Mosesso, Lorenzo; Tomarchio, Luca; Bhattarai, Niraj; Macis, Salvatore; Gori, Paola; Grilli, Antonio; Cestelli Guidi, Mariangela; Philip, John; Pulci, Olivia; Lupi, Stefano. - In: NANOSCALE ADVANCES. - ISSN 2516-0230. - (2024), pp. 1-8. [10.1039/d4na00737a]
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11573/1725624
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