Achieving a strong and robust chiral response in plasmonic metasurfaces is among the key goals of current nanophotonic research. In this work, we theoretically show that the circular dichroism (CD) of a metal metasurface can be maximized by exploiting the concept of a bound state in a continuum (BIC) with symmetry breaking. We consider a gold metasurface with a deformation of circular holes into oval holes. The chiral response at small values of the angle of incidence is dominated by a quasi-BIC, with nearly maximal values of the absorption CD that are almost independent of the deformation. A strong CD in emission is also demonstrated. Symmetry analysis and mode profiles show that the extrinsically chiral response does indeed follow from a symmetry-broken BIC and is associated with a strong enhancement of the local electrical field. The concept of a plasmonic BIC with symmetry breaking provides a robust pathway to increase the chiral response in metal metasurfaces and opens research opportunities in chiral plasmonics that combine narrow resonances with local field enhancement.

Maximum Chirality Empowered by a Bound State in a Continuum in a Plasmonic Metasurface / Ali, Hanan; Zanotti, Simone; Pellegrini, Giovanni; Petronijevic, Emilija; Andreani, Lucio Claudio. - In: ACS APPLIED OPTICAL MATERIALS. - ISSN 2771-9855. - 2:5(2024), pp. 825-833. [10.1021/acsaom.4c00097]

Maximum Chirality Empowered by a Bound State in a Continuum in a Plasmonic Metasurface

Petronijevic, Emilija;
2024

Abstract

Achieving a strong and robust chiral response in plasmonic metasurfaces is among the key goals of current nanophotonic research. In this work, we theoretically show that the circular dichroism (CD) of a metal metasurface can be maximized by exploiting the concept of a bound state in a continuum (BIC) with symmetry breaking. We consider a gold metasurface with a deformation of circular holes into oval holes. The chiral response at small values of the angle of incidence is dominated by a quasi-BIC, with nearly maximal values of the absorption CD that are almost independent of the deformation. A strong CD in emission is also demonstrated. Symmetry analysis and mode profiles show that the extrinsically chiral response does indeed follow from a symmetry-broken BIC and is associated with a strong enhancement of the local electrical field. The concept of a plasmonic BIC with symmetry breaking provides a robust pathway to increase the chiral response in metal metasurfaces and opens research opportunities in chiral plasmonics that combine narrow resonances with local field enhancement.
2024
plasmonic metasurfaces; bound states in a continuum; symmetry breaking; extrinsic chirality; circular dichroism
01 Pubblicazione su rivista::01a Articolo in rivista
Maximum Chirality Empowered by a Bound State in a Continuum in a Plasmonic Metasurface / Ali, Hanan; Zanotti, Simone; Pellegrini, Giovanni; Petronijevic, Emilija; Andreani, Lucio Claudio. - In: ACS APPLIED OPTICAL MATERIALS. - ISSN 2771-9855. - 2:5(2024), pp. 825-833. [10.1021/acsaom.4c00097]
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11573/1717328
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