Anomalous-diffusion, the departure of the spreading dynamics of diffusing particles from the traditional law of Brownian-motion, is a signature feature of a large number of complex soft-matter and biological systems. Anomalous-diffusion emerges due to a variety of physical mechanisms, e.g., trapping interactions or the viscoelasticity of the environment. However, sometimes systems dynamics are erroneously claimed to be anomalous, despite the fact that the true motion is Brownian-or vice versa. This ambiguity in establishing whether the dynamics as normal or anomalous can have far-reaching consequences, e.g., in predictions for reaction- or relaxation-laws. Demonstrating that a system exhibits normal- or anomalous-diffusion is highly desirable for a vast host of applications. Here, we present a criterion for anomalous-diffusion based on the method of power-spectral analysis of single trajectories. The robustness of this criterion is studied for trajectories of fractional-Brownian-motion, a ubiquitous stochastic process for the description of anomalous-diffusion, in the presence of two types of measurement errors. In particular, we find that our criterion is very robust for subdiffusion. Various tests on surrogate data in absence or presence of additional positional noise demonstrate the efficacy of this method in practical contexts. Finally, we provide a proof-of-concept based on diverse experiments exhibiting both normal and anomalous-diffusion.Anomalous-diffusion identifies the departure of diffusive dynamics from the traditional Brownian-motion and is a signature feature of a large number of complex soft-matter and biological systems. This article reports an analysis of an easy to implement method to decide on the type of an apparent anomaly, even in the presence of localisation errors.

Towards a robust criterion of anomalous diffusion / Sposini, V; Krapf, D; Marinari, E; Sunyer, R; Ritort, F; Taheri, F; Selhuber-Unkel, C; Benelli, R; Weiss, M; Metzler, R; Oshanin, G. - In: COMMUNICATIONS PHYSICS. - ISSN 2399-3650. - 5:1(2022). [10.1038/s42005-022-01079-8]

Towards a robust criterion of anomalous diffusion

Krapf, D;Marinari, E;Ritort, F;
2022

Abstract

Anomalous-diffusion, the departure of the spreading dynamics of diffusing particles from the traditional law of Brownian-motion, is a signature feature of a large number of complex soft-matter and biological systems. Anomalous-diffusion emerges due to a variety of physical mechanisms, e.g., trapping interactions or the viscoelasticity of the environment. However, sometimes systems dynamics are erroneously claimed to be anomalous, despite the fact that the true motion is Brownian-or vice versa. This ambiguity in establishing whether the dynamics as normal or anomalous can have far-reaching consequences, e.g., in predictions for reaction- or relaxation-laws. Demonstrating that a system exhibits normal- or anomalous-diffusion is highly desirable for a vast host of applications. Here, we present a criterion for anomalous-diffusion based on the method of power-spectral analysis of single trajectories. The robustness of this criterion is studied for trajectories of fractional-Brownian-motion, a ubiquitous stochastic process for the description of anomalous-diffusion, in the presence of two types of measurement errors. In particular, we find that our criterion is very robust for subdiffusion. Various tests on surrogate data in absence or presence of additional positional noise demonstrate the efficacy of this method in practical contexts. Finally, we provide a proof-of-concept based on diverse experiments exhibiting both normal and anomalous-diffusion.Anomalous-diffusion identifies the departure of diffusive dynamics from the traditional Brownian-motion and is a signature feature of a large number of complex soft-matter and biological systems. This article reports an analysis of an easy to implement method to decide on the type of an apparent anomaly, even in the presence of localisation errors.
2022
diffusion "anomalous diffusion" "brownian motion"
01 Pubblicazione su rivista::01a Articolo in rivista
Towards a robust criterion of anomalous diffusion / Sposini, V; Krapf, D; Marinari, E; Sunyer, R; Ritort, F; Taheri, F; Selhuber-Unkel, C; Benelli, R; Weiss, M; Metzler, R; Oshanin, G. - In: COMMUNICATIONS PHYSICS. - ISSN 2399-3650. - 5:1(2022). [10.1038/s42005-022-01079-8]
File allegati a questo prodotto
Non ci sono file associati a questo prodotto.

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11573/1680176
 Attenzione

Attenzione! I dati visualizzati non sono stati sottoposti a validazione da parte dell'ateneo

Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 11
  • ???jsp.display-item.citation.isi??? 9
social impact