Using low-temperature scanning tunneling spectroscopy, we map the local density of states of graphene quantum dots supported on Ir(111). Because of a band gap in the projected Ir band structure around the graphene K point, the electronic properties of the QDs are dominantly graphenelike. Indeed, we compare the results favorably with tight binding calculations on the honeycomb lattice based on parameters derived from density functional theory. We find that the interaction with the substrate near the edge of the island gradually opens a gap in the Dirac cone, which implies soft-wall confinement. Interestingly, this confinement results in highly symmetric wave functions. Further influences of the substrate are given by the known moire potential and a 10% penetration of an Ir surface resonance into the graphene layer.

Wave-Function Mapping of Graphene Quantum Dots with Soft Confinement / Subramaniam, D; Libisch, F; Li, Y; Pauly, C; Geringer, V; Reiter, R; Mashoff, T; Liebmann, M; Burgdorfer, J; Busse, C; Michely, T; Mazzarello, R; Pratzer, M; Morgenstern, M. - In: PHYSICAL REVIEW LETTERS. - ISSN 0031-9007. - 108:4(2012). [10.1103/PhysRevLett.108.046801]

Wave-Function Mapping of Graphene Quantum Dots with Soft Confinement

Mazzarello R;
2012

Abstract

Using low-temperature scanning tunneling spectroscopy, we map the local density of states of graphene quantum dots supported on Ir(111). Because of a band gap in the projected Ir band structure around the graphene K point, the electronic properties of the QDs are dominantly graphenelike. Indeed, we compare the results favorably with tight binding calculations on the honeycomb lattice based on parameters derived from density functional theory. We find that the interaction with the substrate near the edge of the island gradually opens a gap in the Dirac cone, which implies soft-wall confinement. Interestingly, this confinement results in highly symmetric wave functions. Further influences of the substrate are given by the known moire potential and a 10% penetration of an Ir surface resonance into the graphene layer.
2012
01 Pubblicazione su rivista::01a Articolo in rivista
Wave-Function Mapping of Graphene Quantum Dots with Soft Confinement / Subramaniam, D; Libisch, F; Li, Y; Pauly, C; Geringer, V; Reiter, R; Mashoff, T; Liebmann, M; Burgdorfer, J; Busse, C; Michely, T; Mazzarello, R; Pratzer, M; Morgenstern, M. - In: PHYSICAL REVIEW LETTERS. - ISSN 0031-9007. - 108:4(2012). [10.1103/PhysRevLett.108.046801]
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11573/1465708
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