The recent advent of free-electron laser (FEL) sources is driving the scientific community to extend table-top laser research to shorter wavelengths adding elemental selectivity and chemical state specificity. Both a compact setup (mini-TIMER) and a separate instrument (EIS-TIMER) dedicated to four-wave-mixing (FWM) experiments has been designed and constructed, to be operated as a branch of the Elastic and Inelastic Scattering beamline: EIS. The FWM experiments that are planned at EIS-TIMER are based on the transient grating approach, where two crossed FEL pulses create a controlled modulation of the sample excitations while a third time-delayed pulse is used to monitor the dynamics of the excited state. This manuscript describes such experimental facilities, showing the preliminary results of the commissioning of the EIS-TIMER beamline, and discusses original experimental strategies being developed to study the dynamics of matter at the fs-nm time-length scales. In the near future such experimental tools will allow more sophisticated FEL-based FWM applications, that also include the use of multiple and multi-color FEL pulses.
Experimental setups for FEL-based four-wave mixing experiments at FERMI / Bencivenga, F., Zangrando, M., Svetina, C., Abrami, A., Battistoni, A., Borghes, R., Capotondi, F., Cucini, R., Dallari, F., Danailov, M., Demidovich, A., Fava, C., Gaio, G., Gerusina, S., Gessini, A., Giacuzzo, F., Gobessi, R., Godnig, R., Grisonich, R., Kiskinova, M., et al.. - In: JOURNAL OF SYNCHROTRON RADIATION. - ISSN 1600-5775. - 23:1(2016), pp. 132-40-140. [10.1107/S1600577515021104]
Experimental setups for FEL-based four-wave mixing experiments at FERMI
Rago, Ilaria;
2016
Abstract
The recent advent of free-electron laser (FEL) sources is driving the scientific community to extend table-top laser research to shorter wavelengths adding elemental selectivity and chemical state specificity. Both a compact setup (mini-TIMER) and a separate instrument (EIS-TIMER) dedicated to four-wave-mixing (FWM) experiments has been designed and constructed, to be operated as a branch of the Elastic and Inelastic Scattering beamline: EIS. The FWM experiments that are planned at EIS-TIMER are based on the transient grating approach, where two crossed FEL pulses create a controlled modulation of the sample excitations while a third time-delayed pulse is used to monitor the dynamics of the excited state. This manuscript describes such experimental facilities, showing the preliminary results of the commissioning of the EIS-TIMER beamline, and discusses original experimental strategies being developed to study the dynamics of matter at the fs-nm time-length scales. In the near future such experimental tools will allow more sophisticated FEL-based FWM applications, that also include the use of multiple and multi-color FEL pulses.| File | Dimensione | Formato | |
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